RESUMEN
Generation of coherent light with desirable amplitude and phase profiles throughout the optical spectrum is a key issue in optical technologies. Nonlinear wavefront shaping offers an exceptional way to achieve this goal by converting an incident light beam into the beam (or beams) of different frequency with spatially modulated amplitude and phase. The realization of such frequency conversion and shaping processes critically depends on the matching of phase velocities of interacting waves, for which nonlinear photonic crystals (NPCs) with spatially modulated quadratic nonlinearity have shown great potential. Here, we present the first experimental demonstration of nonlinear wavefront shaping with three-dimensional (3D) NPCs formed by ultrafast-light-induced ferroelectric domain inversion approach. Compared with those previously used low-dimensional structures, 3D NPCs provide all spatial degrees of freedom for the compensation of phase mismatch in nonlinear interactions and thereby constitute an unprecedented system for the generation and control of coherent light at new frequencies.
RESUMEN
We present an experimental study on the Cerenkov second harmonic emission in a novel sunflower spiral array of ferroelectric domains in LiNbO3 crystal. The spiral patterns offer a diffusive, circularly symmetric distribution of reciprocal lattice vectors, thereby enabling enhanced emission of the Cerenkov beam in a broad spectral range. Instead of the traditional electric field poling, the sunflower spiral patterns are fabricated here by using our pioneering method of ferroelectric domain engineering with ultrafast light. This all-optical method gives access to high quality domain structures with short periods, which is beneficial for efficient Cerenkov harmonic generation.
RESUMEN
We report the development of microscopic size gradient index vortex masks using the modified stack-and-draw technique. The vortex mask has a form of flat surface all-glass plate. Its functionality is determined by an internal nanostructure composed of two types of soft glass nanorods. The generation of optical vortices with charges 1 and 2 is demonstrated.
RESUMEN
We introduce a custom-cut periodically poled ferroelectric crystal for the phase matching of multistep cascading frequency conversion processes. Our approach involves combination of collinear second harmonic generation and transverse sum frequency mixing via the total internal reflection of the fundamental and collinear second harmonic beams. As a proof of concept we demonstrate multiple frequency generation with an enhanced fourth harmonic signal in a one-dimensional periodically poled LiNbO3 crystal.
RESUMEN
We report Raman spectra measurements on a MoS(2) monolayer supported on SiO(2) as a function of temperature. Unlike in previous studies, the positions of the two main Raman modes, E(2g)(1) and A(1g) exhibited nonlinear temperature dependence. Temperature dependence of phonon shifts and widths is explained by optical phonon decay process into two acoustic phonons. On the basis of Raman measurements, local temperature change under laser heating power at different global temperatures is derived. Obtained results contribute to our understanding of the thermal properties of two-dimensional atomic crystals and can help to solve the problem of heat dissipation, which is crucial for use in the next generation of nanoelectronic devices.
